• Login
    View Item 
    •   NM-AIST Home
    • Materials, Energy, Water and Environmental Sciences
    • Research Articles
    • View Item
    •   NM-AIST Home
    • Materials, Energy, Water and Environmental Sciences
    • Research Articles
    • View Item
    JavaScript is disabled for your browser. Some features of this site may not work without it.

    Mitigation of Fluoride Contamination in Drinking Water Supply Sources by Adsorption Using Bone Char: Effects of Mineral and Organic Matrix

    Thumbnail
    View/Open
    Full text (6.828Mb)
    Date
    2024-10-20
    Author
    Ibrahim, Mohamed
    Oyetade, Joshua
    Dalhatou, Sadou
    Nikiforov, Anton
    Leys, Christophe
    Hilonga, Askwar
    Metadata
    Show full item record
    Abstract
    This study focused on fluoride (F−) contamination of water sources in Bahimi village, Cameroon. After the first investigation, results revealed that all water samples collected had elevated concentrations of fluoride ions (2.3 ± 0.1) mg/L to (4.5 ± 0.2) mg/L above the WHO guidelines (less than 1.5 mg/L). To mitigate the F− levels, the use of bone char (BC) as an adsorbent material was proposed and its performance was tested. BC was prepared from bovine bones at different calcination temperatures (350 °C, 450 °C, 550 °C and 650 °C) and residence times (1 h and 2 h). The prepared materials were characterized in detail by SEM/EDS, BET, FTIR, and XRD. The BET findings indicated that the surface area of BC samples decreased with increasing calcination temperature and residence time. At a lower heating temperature and holding time (350 °C, 1 h), the prepared BC exhibited a higher specific surface area (112.3 ± 0.3) m2/g and adsorption capacity for F− in the sampled water. Also, the batch adsorption experiments showed that the optimized adsorbent dose of 8 g/L facilitates the reduction in the F− level of the sampled water below the acceptable limit level (1.5 mg/L) within 5 min of treatment. The presence of Ca2+ and Mg2+ in natural water has a positive effect on the removal of F− in BC resulting in a high adsorption performance range of (72.5 ± 1.4)% to (80.3 ± 0.6)%. It was found that the adsorption of Ca2+ on the BC surface occurs via cation exchange with Na+. However, an increase in dissolved organic carbon (DOC) in the treated water limited the application of BC. Overall, the study presented a cost-effective adsorbent for the removal of this recalcitrant ion in the water source.
    URI
    https://doi.org/10.3390/w16202991
    https://dspace.nm-aist.ac.tz/handle/20.500.12479/2903
    Collections
    • Research Articles

    Nelson Mandela-AIST copyright © 2021  DuraSpace
    Theme by 
    Atmire NV
     

     

    Browse

    All PublicationsCommunities & CollectionsBy Issue DateAuthorsTitlesSubjectsThis CollectionBy Issue DateAuthorsTitlesSubjects

    My Account

    LoginRegister

    Nelson Mandela-AIST copyright © 2021  DuraSpace
    Theme by 
    Atmire NV